Among 203 counties EPA currently lists as nonattainment for ozone or fine particles, the largest are Los Angeles County, CA (10,013,976 residents), Cook County, IL and Harris County, TX.
What it shows: Los Angeles County, CA is the largest at 10,013,976, followed by Cook County, IL at 5,275,555; the smallest shown is Queens County, NY at 2,405,425.
Data and chart by CalcScrape: Emissions Test Cost Calculator